ChemInform Abstract: Ab initio Study of Phosphorus Ion Complexes of Ammonia and Water.
- LOPEZ, X. 1
- UGALDE, J. M. 1
- COSSIO, F. P. 1
- LECEA, B. 1
- LARGO, A. 1
- BARRIENTOS, C. 1
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1
Universidad del País Vasco/Euskal Herriko Unibertsitatea
info
Universidad del País Vasco/Euskal Herriko Unibertsitatea
Lejona, España
ISSN: 0931-7597
Any de publicació: 2010
Volum: 24
Número: 52
Pàgines: no-no
Tipus: Article
Altres publicacions en: ChemInform
Resum
dy of Phosphorus Ion Complexes of Ammonia andWater. — By ab initio calculations for the P(NH3)+ n, P(OH2)+ n (n= 1, 2) and P(NH3)(OH2)+ ion-molecule complexes, optimum geometries(HF/6-31G** and MP2/6-31G*), binding energies (at different levels of theory)and Mulliken charges are determined. The binding energies for the oneligand complexes are larger than those expected from an electrostatic bindingmechanism. This is ascribed to some electron dative bonding character. Forthe two-ligand complexes binding energies closer to the electrostatic ones areobtained indicating a higher electrostatic character than that of the one-ligandcomplexes.
Referències bibliogràfiques
- LOPEZ, (1993), J. Phys. Chem., 97, pp. 9337, 10.1021/j100139a014